'Waking up' with Sam Harris is filled with fabulous interviews.
Not all of them are centered on atheism, in fact very few are actually.

Some of my recent favorites:
- Robert Sapolsky on 'The biology of good and evil'. How much free will do we really have?
- Gavin de Becker on 'Living with violence'. Some great advice if you are ever in a dangerous situation.
- Mark Bowden on 'Must accept a nuclear N. Korea'. Great insight on the options (or lack thereof) re: North Korea.
- Tristan Harris on 'What is technology doing to us'. Do computer scientists need a hypocratic oath?
- Garry Kasparov on 'The Putin question'. What is uncle Vlad up to?